Acknowledgement
This work was sponsored by the Nuclear R&D program of the Korean Ministry of Science and ICT (2017M2A8A5015077).
References
- C.E. Stevenson, The EBR-II Fuel Cycle Story, 53-198, La Grange park, Illinois (1987).
- H. Lee, G.I. Park, K.H. Kang, J.M. Hur, J.G. Kim, D.H. Ahn, Y.Z. Cho, and E.H. Kim, "Pyroprocessing Technology Development at KAERI", Nucl. Eng. Technol., 43(4), 317-328 (2011). https://doi.org/10.5516/NET.2011.43.4.317
- S.D. Herrmann, S.X. Li, M.F. Simpson, and S. Phongikaroon, "Electrolytic Reduction of Spent Nuclear Oxide Fuels as Part of an Integral Process to Separate and Recover Actinides From Fission Products", Sep. Sci. Technol., 41(10), 1965-1983 (2006). https://doi.org/10.1080/01496390600745602
- Y. Sakamura and T. Omori, "Electrolytic Reduction and Electrorefining of Uranium to Develop Pyrochemical Reprocessing of Oxide Fuels", Nucl. Technol., 171(3), 266-275 (2010). https://doi.org/10.13182/nt10-a10861
- E.Y. Choi, J. Lee, D.H. Heo, S.K. Lee, M.K. Jeon, S.S. Hong, S.W. Kim, H.W. Kang, S.C. Jeon, and J.M. Hur, "Electrolytic Reduction Runs of 0.6 kg Scale-Simulated Oxide Fuel in a Li2O-LiCl Molten Salt Using Metal Anode Shrouds", J. Nucl. Mater., 489, 1-8 (2017). https://doi.org/10.1016/j.jnucmat.2017.03.035
- W. Park, E.Y. Choi, S.W. Kim, S.C. Jeon, Y.H. Cho, and J.M. Hur, "Electrolytic Reduction of a Simulated Oxide Spent Fuel and the Fates of Representative Elements in a Li2O-LiCl Molten Salt", J. Nucl. Mater., 477, 59-66 (2016). https://doi.org/10.1016/j.jnucmat.2016.04.058
- S.K. Lee, M.K. Jeon, S.W. Kim, E.Y. Choi. J. Lee, S.S. Hong, S.C. Oh, and J.M. Hur, "Evaluation of Pt Anode Stability in Repeated Electrochemical Oxide Reduction Reactions for Pyroprocessing", J. Radioanal. Nucl. Chem., 316(3), 1053-1058 (2018). https://doi.org/10.1007/s10967-018-5765-9
- J.M. Hur, J.S. Cha, and E.Y. Choi, "Can Carbon be an Anode for Electrochemical Reduction in a LiCl-Li2O Molten Salt?", ECS Electrochem. Lett., 3(10), E5-E7 (2014). https://doi.org/10.1149/2.0071410eel
- H.Y. Ryu, S.M. Jeong, Y.C. Kang, and J.G. Kim, "Electrochemical Carbon Formation From a Graphite Anode in Li2O/LiCl Molten Salt", Asian J. Chem., 25(12), 7019-7022 (2013). https://doi.org/10.14233/ajchem.2013.08
- S.W. Kim, M.K. Jeon, H.W. Kang, S.K. Lee, E.Y. Choi, W. Park, S.S. Hong, S.C. Oh, and J.M. Hur, "Carbon Anode With Repeatable Use of LiCl Molten Salt for Electrolytic Reduction in Pyroprocessing", J. Radioanal. Nucl. Chem., 310(1), 463-467 (2016). https://doi.org/10.1007/s10967-016-4786-5
- S.W. Kim, D.H. Heo, S.K. Lee, M.K. Jeon, W. Park, J.M. Hur, S.S. Hong, S.C. Oh, and E.Y. Choi, "A Preliminary Study of Pilot-Scale Electrolytic Reduction of UO2 Using a Graphite Anode", Nucl. Eng. Technol., 49(7), 1451-1456 (2017). https://doi.org/10.1016/j.net.2017.05.004
- E. Nakamura, H. Takata, Y. Yokoyama, and H. Miyamoto, Process for producing metallic lithium, US patent No. 8,911,610 B2 (2014).
- D.R. Lide, CRC Handbook of Chemistry and Physics, Internet version 2006, 4-70, Taylor and Francis, Boca Raton, FL (2006).
- J.W. Kim and H.G. Lee, "Thermal and Carbothermic Decomposition of Na2CO3 and Li2CO3", Metall. Mater. Trans. B, 32(1), 17-24 (2001). https://doi.org/10.1007/s11663-001-0003-0