DOI QR코드

DOI QR Code

On-Site Treatment of Soil Contaminated by Heavy Metals and Petroleum using Relocatable Soil Washing Equipment

  • Received : 2019.12.15
  • Accepted : 2019.12.25
  • Published : 2020.03.31

Abstract

We studied the on-site treatment of soil contaminated by heavy metals and petroleum was tested using relocatable soil washing equipment for greater remediation efficiency. Different combinations of pH and solid/liquid ratio were tested to determine the optimum balance, settling on values of 5 and 1:2, respectively. Next, soils containing Pb, Hg, and petroleum were further tested to assess the optimum number of washing cycles. The remediation efficiency of Pb and Hg in soil contaminated solely by heavy metals was 90.1% and 86.4% after three and two washings, respectively. The remediation efficiency of petroleum in soil contaminated solely by petroleum was 98.8% after one washing. When soil contaminated by both heavy metals and petroleum was cleaned, up to 91.0% of Pb, 86.9% of Hg, and 96.1% of petroleum was removed after two, one, and one washings, respectively. We conducted all remediation efficiencies and concentration reductions satisfied the standard threshold for soil contamination in South Korea.

Keywords

References

  1. C. Adam, B. Peplinski, M. Michaelis, G. Kley and F.G. Simon, "Thermochemical treatment of sewage sludge ashes for phosphorus recovery", Waste Management, vol. 29, pp. 1122-1128, March 2009. DOI: https://doi.org/10.1016/j.wasman.2008.09.011
  2. D. Huguenot, E. Mousset, E.D. van Hullebusch and M.A. Oturan, "Combination of surfactant enhanced soil washing and electro-Fenton process for the treatment of soils contaminated by petroleum hydrocarbons", Journal of Environmental Management, vol. 153, pp. 40-47. April 2015. DOI: https://doi.org/10.1016/j.jenvman.2015.01.037
  3. Ministry of Environment, "Soil clean-up of industrial development for the standardization and competitive advantage", Government of South Korea, pp. 85, 2010.
  4. J.C. Tang, X.Q. Lu, Q. Sun and W.Y. Zhu, "Aging effect of petroleum hydrocarbons in soil under different attenuation conditions", Agriculture Ecosystems and Environment, vol. 149, pp. 109-117, March 2012. DOI: https://doi.org/10.1016/j.agee.2011.12.020
  5. M.A. Mohamed, A. Efligenir, J. Husson, J. Persello, P. Fievet and N. Fatin-Rouge, "Extraction of heavy metals from a contaminated soil by reusing chelating agent solutions", Journal of Environmental Engineering, vol. 1, no. 3, pp. 363-368, September 2013. DOI: https://doi.org/10.1016/j.jece.2013.05.015
  6. M. Jelusic and D. Lestan, "Effect of EDTA washing of metal polluted garden soils. Part I: Toxicity hazards and impact on soil properties", Science of the Total Environment, vol. 475, pp. 132-141, March 2014. DOI: https://doi.org/10.1016/j.scitotenv.2013.11.049
  7. X. Zhang, Z. Liu, Q. Yu, N.T. Luc, Y. Bing, B. Zhu and W. Wang, "Effect of petroleum on decomposition of shrubgrass litters in soil in Northern Shanxi of China", Journal of Environment Science, vol. 33, pp. 245-253, July 2015. DOI: https://doi.org/10.1016/j.jes.2014.12.013
  8. T. Sabbas, A. Polettini, R. Pomi, T. Astrup, O. Hjelmar, P. Mostbauer, G. Cappai, G. Magel, S. Salhofer, C. Speiser, S. Heuss-Assbichler, R. Klein and P. Lechner, "Management of municipal solid waste incineration residues", Waste Management, vol. 23, pp. 61-88, July 2003. DOI: https://doi.org/10.1016/S0956-053X(02)00161-7
  9. J. Hyks, I. Nesterov, E. Mogensen, P. Jensen and T. Astrup, "Leaching from waste incineration bottom ashes treated in a rotary kiln", Waste Management and Research, vol. 29, no. 10, pp. 995-1007, September 2011. DOI: https://doi.org/10.1177/0734242X11417490
  10. K.H. Kim, J.S. Park, H.K. Kim and S.I. Choi, "Optimum management plan for soil contamination facilities", Journal of Soil Science and Fertilizer, vol. 45, no. 2, pp. 293-300, April 2012.
  11. B.L. Lim, "Evaluation of soil washing technology for the remediation of heavy metal contaminated soil", M.D. Thesis, Kyunghee University, Korea, 2005.
  12. C.S. Paek, J.H. Hyun, M.Y. Cho and S.J. Kim, "Remediation of heavy metal contaminated soil by washing process", Journal of Soil Groundwater Environment, vol. 5, no. 1, pp. 45-54, April 2000.
  13. Ministry of Environment, "Official test method soil pollution", Government of South Korea, pp. 63, 2011.
  14. S.A. Zheng, X.Q. Zheng and C. Chen, "Transformation of metal speciation in purple soil as affected by waterlogging", International Journal of Environmental Science and Technology, vol. 10, no. 2, pp. 351-358, December 2013. DOI: https://doi.org/10.1007/s13762-012-0146-3
  15. D.C. Cheong, J.H. Lee and S.I. Choi, "Application of soil washing technology to the soil contaminated by heavy metals", Journal of Soil and Groundwater Environment, vol. 2, no. 2, pp. 53-60, September 1997.
  16. D.H. Lee, I.W. Na and K.Y. Hwang, "Soil remediation using soil washing system in hydrocarbon contaminated field", Journal of Economic and Environmental Geology, vol. 35, no. 4, pp. 369-372, March 2002.
  17. C.D. Lee, J.C. Yoo, J.S. Yang, J. Kong and K.T. Back, "Extraction of total petroleum hydrocarbons from petroleum oil-contaminated sandy soil by soil washing", Journal of Soil and Groundwater Environment, vol. 18, no. 7, pp. 18-24, December 2013. https://doi.org/10.7857/JSGE.2013.18.7.018
  18. J.H. Kim, "On-site treatment of the petroleum oil and heavy metals contaminated soil using soil washing technique", M.D. Thesis, Seoul National University of Science and Technology, Korea, 2015.
  19. H.J. Choi, "Cleanup of soil contaminated with combined pollutants by soil washing", Ph.D. Thesis, Korea University, Korea, 2006.
  20. S.J. Choi, "A study on the remediation of lead contaminated-soils at clay pigeon shooting range by soil washing", M.D. Thesis, Inha University, Korea, 2008.
  21. T.S. Rӧtting, M. Mercado, M.E. García and J. Quintanilla, "Environmental distribution and health impacts of As and Pb in crops and soils near Vinto smelter, Oruro, Bolivia", International Journal of Environmental Science and Technology, vol. 11, no. 4, pp. 935-948, May 2014. DOI: https://doi.org/10.1007/s13762-013-0313-1
  22. G. Ludajic, L. Pezo, N. Filipovic and J. Filipovic, "A chemometric approach to study the effects of motorway proximity on microelements content in wheat and soil", International Journal of Environmental Science and Technology. vol. 12, no. 8, pp. 2639-2648, October 2015. DOI: https://doi.org/10.1007/s13762-014-0673-1
  23. M.J. Kim, "A study on removal of heavy metals (Cu, Zn, and Pb) from contaminated soil by soil washing", Journal of Economic and Environmental Geology, Vol. 46, No. 6, pp. 509-520, December 2013. DOI: https://doi.org/10.9719/EEG.2013.46.6.509
  24. M.H. Lee, J.H. Chen, I.S. Kim, H.M. Kang and S.K. Kim, "Chemical soil washing using hydrogen peroxide for oil contaminated soils in batch tests". Journal of Atmospheric Environment, vol. 41, no. 3, pp. 2505-2508, May 2007.
  25. J.H. Hwang, S.K. Kim, S,H. Ha, B.H. Son and K.J. Oh, " The empirical study NaOH/$H_2O_2$-Enhanced soil washing by a treatment conditions to remediate petroleum contaminated site", Journal of Environmental Engineering, vol. 1, pp. 1513-1515, May 2007.
  26. I.R. Jang, "Treatment of heavy metal and total petroleum hydrocarbon by soil washing", M.D. Thesis, Ulsan University, Korea, 2010.
  27. H.J. Shin, M.H. Oh and J.B. Park, "Evaluation of newly developed Lab-Scale soil washing equipment for fine-grain soil", Journal of Civil Engineering, vol. 66, no. 7, pp. 1609-1610, October 2014.
  28. M.S. Seol, "A study on the remediation of heavy metals contaminated soil using the phytoremediation and soil washing", Ph.D. Thesis, Chosun University, Korea, 2011.
  29. M.H. Chun, H.J. Son and C. Kim, "A study on the isolation of the oil-degradation microbes and treatment efficiency in the oil contaminated soil with peat moss", Journal of Environmental Health, vol. 43, no. 4, pp. 462-469, October 2007.