Journal of Industrial and Engineering Chemistry

  • 제67권
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  • Pages.373-379
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  • 2018
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  • 1226-086X(pISSN)
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  • 1876-794X(eISSN)
한국공업화학회 (The Korean Society of Industrial and Engineering Chemistry)
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DOI QR코드

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Fabrication of triazine-based Porous Aromatic Framework (PAF) membrane with structural flexibility for gas mixtures separation

  • Wang, Lei (Key Laboratory of Polyoxometalate Science of the Ministry of Education, Faculty of Chemistry, Northeast Normal University) ;
  • Jia, Jiangtao (State Key Laboratory of Inorganic Synthesis and Preparative Chemistry, College of Chemistry, Jilin University) ;
  • Faheem, Muhammad (Key Laboratory of Polyoxometalate Science of the Ministry of Education, Faculty of Chemistry, Northeast Normal University) ;
  • Tian, Yuyang (Key Laboratory of Polyoxometalate Science of the Ministry of Education, Faculty of Chemistry, Northeast Normal University) ;
  • Zhu, Guangshan (Key Laboratory of Polyoxometalate Science of the Ministry of Education, Faculty of Chemistry, Northeast Normal University)
  • 투고 : 2018.04.19
  • 심사 : 2018.07.07
  • 발행 : 2018.11.25
⟨ 이전 논문 다음 논문 ⟩

초록

A transparent, freestanding Porous Aromatic Framework-97 (PAF-97) membrane was successfully synthesized via a one-step acid-catalyzed reaction. Due to the introduction of ether groups, the obtained PAF-97 membrane possesses enhanced structural flexibility, thus increasing the flexibility of the resulting membrane. This is proofed by the fact that the feeding pressure of the membrane reaches as high as 5.5 bar during the separation of gas mixtures. The Young's moduli of the membrane were 6.615 GPa and 11.11 GPa, either in a dry or hydrated state respectively. To be highlighted, under a feeding pressure of 3.6 bar, the PAF-97 membrane rendered the permeance values of $2.90{\times}10^{-7}$, $1.29{\times}10^{-8}mol\;m^{-2}s^{-1}Pa^{-1}$ for $CO_2$ and $CH_4$, respectively, with a $CO_2/CH_4$ permselectivity of 22.48.

키워드

과제정보

연구 과제 주관 기관 : National Natural Science Foundation of China (NSFC)

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