Journal of Industrial and Engineering Chemistry

  • Volume 68
  • /
  • Pages.14-23
  • /
  • 2018
  • /
  • 1226-086X(pISSN)
  • /
  • 1876-794X(eISSN)
The Korean Society of Industrial and Engineering Chemistry (한국공업화학회)
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Enhanced photo-Fenton degradation of tetracycline using TiO2-coated α-Fe2O3 core-shell heterojunction

  • Zheng, Xiaogang (College of Chemistry and Chemical Engineering, Neijiang Normal University) ;
  • Fu, Wendi (College of Chemistry and Chemical Engineering, Neijiang Normal University) ;
  • Kang, Fuyan (College of Chemistry and Chemical Engineering, Neijiang Normal University) ;
  • Peng, Hao (College of Chemistry and Chemical Engineering, Yangtz Normal University) ;
  • Wen, Jing (Key Laboratory of Comprehensive and Highly Efficient Utilization of Salt Lake Resources, Key Laboratory of Salt Lake Resources Chemistry of Qinghai Province, Qinghai Institute of Salt Lakes, Chinese Academy of Sciences)
  • Received : 2018.05.30
  • Accepted : 2018.07.19
  • Published : 2018.12.25
⟨ Previous Next ⟩

Abstract

$TiO_2-coated$ cubic ${\alpha}-Fe_2O_3$ with mostly exposed (012) and (101) facets (${\alpha}-Fe_2O_3@TiO_2$) was fabricated using a hydrothermal route for the photo-Fenton degradation of tetracycline under visible light irradiation. $TiO_2$ coating could greatly affect the photocatalytic activity of ${\alpha}-Fe_2O_3@TiO_2$. Compared with cubic ${\alpha}-Fe_2O_3$ alone for photodegradation of tetracycline, ${\alpha}-Fe_2O_3@TiO_2$ with $TiO_2$ shell of around 15 nm exhibited higher removal efficiency of tetracycline in photo-Fenton system, and its durability was slightly affected after five cycle times under same conditions. It is ascribed to the well-matched interface between cubic ${\alpha}-Fe_2O_3$ core and $TiO_2$ shell, leading to the broadened light-absorption and the efficient separation of photo-generated electon-hole pairs. The $^{\bullet}OH$ radicals were main responsible for the advanced photocatalytic performance of ${\alpha}-Fe_2O_3@TiO_2$ in visible-light driven degradation of tetracycline.

Keywords

Acknowledgement

Supported by : National Natural Science Foundation of China

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