한국대기환경학회지 (Journal of Korean Society for Atmospheric Environment)

  • 제33권5호
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  • Pages.458-472
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  • 2017
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  • 1598-7132(pISSN)
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  • 2383-5346(eISSN)
한국대기환경학회 (Korean Society for Atmospheric Environment)
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제주 애월 대기오염집중측정소의 PM2.5 에어로졸 화학성분 자료를 이용한 광학특성 및 직접적 복사강제력 추정 연구

Estimations of the Optical Properties and Direct Radiative Forcing of Aerosol Chemical Components in PM2.5 Measured at Aewol Intensive Air Monitoring Site on Jeju Island

  • 박연희 (제주대학교 해양과학대학 지구해양과학과) ;
  • 송상근 (제주대학교 해양과학대학 지구해양과학과) ;
  • 강창희 (제주대학교 자연과학대학 화학.코스메틱스학과) ;
  • 송정민 (제주대학교 자연과학대학 화학.코스메틱스학과)
  • Park, Yeon-Hee (Department of Earth and Marine Sciences, Jeju National University) ;
  • Song, Sang-Keun (Department of Earth and Marine Sciences, Jeju National University) ;
  • Kang, Chang-Hee (Department of Chemistry and Cosmetics, Jeju National University) ;
  • Song, Jung-Min (Department of Chemistry and Cosmetics, Jeju National University)
  • 투고 : 2017.08.02
  • 심사 : 2017.09.07
  • 발행 : 2017.10.31
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초록

The optical properties and direct aerosol radiative forcing (DARF) of different aerosol components in $PM_{2.5}$ (water-soluble, insoluble, black carbon (BC), and sea-salt) were estimated using the hourly resolution data measured at Aewol intensive air monitoring site on Jeju Island during 2013, based on a modeling approach. In general, the water-soluble component was predominant over all other components with respect to its impact on the optical properties(except for absorbing BC) and DARF. The annual mean aerosol optical depth (AOD) at 500 nm for the water-soluble component was $0.14{\pm}0.14$ ($0.04{\pm}0.01$ for BC). The total DARF at the surface ($DARF_{SFC}$) and top of the atmosphere ($DARF_{TOA}$), and in the atmosphere ($DARF_{ATM}$) for most aerosol components(except for sea-salt) during the daytime were highest in spring and lowest in fall and/or summer. The maximum $DARF_{SFC}$ of most aerosol components occurred around noon (12:00~14:00 LST) during all seasons, while the maximum $DARF_{TOA}$ occurred in the afternoon (13:00~16:00 LST) during most seasons (except for spring). In addition, the estimated $DARF_{SFC}$ and $DARF_{ATM}$ of the water-soluble component were -20 to $-59W/m^2$ and +3.5 to $+14W/m^2$, respectively, while those of BC were -18 to $-29W/m^2$ and +23 to $+37W/m^2$, respectively.

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