DOI QR코드

DOI QR Code

Background Level and Time Series Variation of Atmospheric Radon Concentrations at Gosan Site in Jeju Island

제주도 고산지역의 대기 라돈 배경농도 및 시계열 변동

  • Song, Jung-Min (Department of Chemistry and Cosmetics, Jeju National University) ;
  • Bu, Jun-Oh (Department of Chemistry and Cosmetics, Jeju National University) ;
  • Kim, Won-Hyung (Department of Chemistry and Cosmetics, Jeju National University) ;
  • Kang, Chang-Hee (Department of Chemistry and Cosmetics, Jeju National University) ;
  • Ko, Hee-Jung (Environmental Meteorology Research Division, National Institute of Meteorological Sciences) ;
  • Chambers, S. (Australian Nuclear Science and Technology Organisation)
  • 송정민 (제주대학교 화학.코스메틱스학과) ;
  • 부준오 (제주대학교 화학.코스메틱스학과) ;
  • 김원형 (제주대학교 화학.코스메틱스학과) ;
  • 강창희 (제주대학교 화학.코스메틱스학과) ;
  • 고희정 (국립기상과학원 환경기상연구과) ;
  • Received : 2017.03.06
  • Accepted : 2017.03.24
  • Published : 2017.04.30

Abstract

The background level and timely variation characteristics of atmospheric $^{222}Rn$ concentrations have been evaluated by the real time monitoring at Gosan site of Jeju Island, Korea, during 2008~2015. The average concentration of atmospheric radon was $2,480mBq\;m^{-3}$ for the study period. The cyclic seasonality of radon was characterized such as winter maximum and summer minimum, consistent with the reduction in terrestrial fetch going to summer. On monthly variations of radon, the mean concentration in October was the highest as $3,041mBq\;m^{-3}$, almost twice as that in July ($1,481mBq\;m^{-3}$). The diurnal radon concentrations increased throughout the nighttime approaching to the maximum ($2,819mBq\;m^{-3}$) at around 7 a.m., and then gradually decreased throughout the daytime by the minimum ($2,069mBq\;m^{-3}$) at around 3 p.m. The diurnal radon cycle in winter showed comparatively small amplitude due to little variability in atmospheric mixing depth, conversely, large amplitude was observed in summer due to relatively a big change in atmospheric mixing depth. The cluster back-trajectories of air masses showed that the high radon events occurred by the predominant continental fetch over through Asia continent, and the radon concentrations from China continent were about 1.9 times higher on the whole than those from the North Pacific Ocean. The concentrations of $PM_{10}$ also increased in proportion to the high radon concentrations, showing a good linear correlation between $PM_{10}$ and radon concentrations.

Keywords

References

  1. Almeida, R.M., D.C. Lauria, A.C. Ferreira, and O. Sracek (2004) Groundwater radon, radium and uranium concentrations in Regiao dos Lagos, Rio de Janeiro State, Brazil. Journal of Environmental Radioactivity, 73(3), 323-334. https://doi.org/10.1016/j.jenvrad.2003.10.006
  2. Bonotto, D.M. and P.C. Padron-Armada (2008) Radon and progeny ($^{214}Pb$ and $^{214}Bi$) in urban water-supply systems of Sao Paulo State, Brazil, Applied Geochemistry, 23(10), 2829-2844. https://doi.org/10.1016/j.apgeochem.2008.04.017
  3. Chambers, S., W. Zahorowski, K. Matsumoto, and M. Uematsu (2009) Seasonal variability of radon-derived fetch regions for Sado Island, Japan, based on 3 years of observations: 2002-2004, Atmospheric Environment, 43(2), 271-279. https://doi.org/10.1016/j.atmosenv.2008.09.075
  4. Chambers, S.D., W. Zahorowski, A.G. Williams, J. Crawford, and A.D. Griffiths (2013) Identifying tropospheric baseline air masses at Mauna Loa Observatory between 2004 and 2010 using Radon-222 and back trajectories, Journal of Geophysical Research, 118, 1-13, doi:10.1029/2012JD018212.
  5. Chambers, S.D., C.H. Kang, A.G. Williams, J. Crawford, A.D. Griffiths, K.H. Kim, and W.H. Kim (2016) Improving the representation of cross-boundary transport of anthropogenic pollution in Southeast Asia using Radon-222, Aerosol and Air Quality Research, 16(4), 958-976, doi: 10.4209/aaqr.2015.08.0522.
  6. Chan, S.W., C.W. Lee, and K.C. Tsui (2010) Atmospheric radon in Hong Kong. Journal of Environmental Radioactivity, 101(6), 494-503. https://doi.org/10.1016/j.jenvrad.2010.02.007
  7. Choi, I.C., S.H. Shin, and W.K. Jo (2009) Evaluation of Radon Levels in Various Public-acess Buildings or Underground Facilities, and Their Temporal Variation in Underground Facilities. Journal of Environmental Toxicology, 24(3), 203-211. (in Korean)
  8. Duckworth, F.A. and J.S. Sandberg (1954) The effect on cities upon horizontal and vertical temperature gradients, Blletin of the American Meteorological Society, 35, 198-207.
  9. Draxler, R.R. and G.D. Rolph (2013) HYSPLIT (HYbrid Single-Particle Lagrangian Integrated Trajectory) Model access via NOAA ARL READY Website (http://ready.arl.noaa.gov/HYSPLIT_traj.php).
  10. Jamil, K., K.K. Al-Ahmady, Fazal-ur-Rehman, S. Ali, A.A. Qureshi, and H.A. Kahn (1997) Relative performance of different types of passive dosimeters employing solid state nuclear track detectors, Health Physics, 73(4), 629-632. https://doi.org/10.1097/00004032-199710000-00006
  11. Kang, C.H., W.H. Kim, C.G. Hu, and D.H. Kang (2012) Real-time monitoring of radon background level at Gosan site, Jeju Island. Journal of Analytical Science & Technology, 25(1), 7-13. (in Korean with English abstract) https://doi.org/10.5806/AST.2012.25.1.007
  12. Kim, E.H., P.S. Kim, C.Y. Kim, K.S. Lee, and K.D. Kwon (1985) Determination of the Mixing Height in Seoul by the Radioactivity Measurement of Radon in Air, Bulletin of Environmental Sciences (Research Institute for Environmental Sciences Hanyang University), 6(2), 129-136.
  13. Kim, W.H., H.J. Ko, C.G. Hu, H. Lee, C. Lee, S. Chambers, A.G. Williams, and C.H. Kang (2014) Background Level of Atmospheric Radon-222 Concentrations at Gosan Station, Jeju Island, Korea in 2011, Bulletin of the Korean Chemical Society, 35(4), 1149-1153. https://doi.org/10.5012/bkcs.2014.35.4.1149
  14. Kim, Y.S., C.M. Lee, K.Y. Kim, H.J. Jeon, J.C. Kim, and T. Iida (2007) Time Series Observations of Atmospheric Radon Concentration in Seoul, Korea for an Analysis of Long-Range Transportation of Air Pollutants in the North-East Asia, Korean Journal of Environmental Health Sciences, 33(4), 283-292. https://doi.org/10.5668/JEHS.2007.33.4.283
  15. Ko, H.J., S.H. Sin, C.G. Hu, W.H. Kim, C.H. Kang, D.H. Kang, and S. Chambers (2013) Time-series Variation of Atmospheric Radon Concentrations at Gosan Site, Jeju Island. Journal of Korean Society for Atmospheric Environment, 29(1), 86-96. (in Korean) https://doi.org/10.5572/KOSAE.2013.29.1.86
  16. Lee, K., S. Seo, J. Yoo, S. Oh, M. Kwon, and W. Lee (2016) Factors influencing indoor radon concentration in detached house. Journal of Odor Indoor Environment, 15(2), 93-99. (in Korean) https://doi.org/10.15250/joie.2016.15.2.93
  17. Miles, J. (1988) Development of maps of radon-prone areas using radon measurements in houses. Journal of Hazardous Materials, 61, 53-58.
  18. Moon, K.H., J.S. Kim, J.K. Ahn, H.C. Kim, and H.M. Lee (2009) Long-term Variation of Radon in Granitic Residual Soil at Mt. Guemjeong in Busan, Korea, Jour. Petrol. Soc. Korea, 18(4), 279-291.
  19. Pitari, G., E. Coppari, N. De Luca, and P. Di Carlo (2014) Observations and box model analysis of radon-222 in the atmospheric surface layer at L'Aquila, Italy: March 2009 case study, Environmental Earth Sciences, 71(5), 2353-2359. https://doi.org/10.1007/s12665-013-2635-1
  20. Vinson, D., T.R. Campbell, and A. Vengosh (2008) Radon transfer from groundwater used in showers to indoor air, Applied Geochemistry, 23(9), 2676-2685. https://doi.org/10.1016/j.apgeochem.2008.05.021
  21. Whittlestone, S. and W. Zahorowski (1998) Baseline radon detectors for shipboard use: Development and deployment in the First Aerosol Characterization Experiment (ACE 1). Journal of Geophysical Research, 103(D13), 16,743-16,751. https://doi.org/10.1029/98JD00687
  22. WMO/GAW (2001) Global Atmosphere Watch Measurements Guide (No. 143), WMO TD No. 1073.
  23. WMO/GAW (2004) 1st International Expert Meeting on Sources and Measurements of Natural Radionuclides Applied to Climate and Air Quality Studies (No. 155), WMO TD No. 1201.
  24. Zahorowski, W., S.D. Chambers, and A. Henderson-Sellers (2004) Ground based radon-222 observations and their application to atmospheric studies. Journal of Environmental Radioactivity, 76(1-2), 3-33. https://doi.org/10.1016/j.jenvrad.2004.03.033
  25. Zahorowski, W., S. Chambers, T. Wang, C.H. Kang, I. Uno, S. Poon, S.N. Oh, S. Wercqynski, J. Kim, and A. Henderson-Sellers (2005) Radon-222 in boundary layer and free tropospheric continental outflow events at three ACE-Asia sites, Tellus, 57(2), 124-140. https://doi.org/10.3402/tellusb.v57i2.16776
  26. Zoran, M.A., M.R. Dida, A.T. Zoran, L.F. Zoran, and A. Dida (2013) Outdoor $^{222}Radon$ concentrations monitoring in relation with particulate matter levels and possible health effects. Journal of Radioanalytical Nuclear Chemistry, 296(3), 1179-1192. https://doi.org/10.1007/s10967-012-2259-z