Numerical Analysis of Electromagnetic and Temperature Fields Induced by Femtosecond Laser Irradiation of Silver Nanowires

은 나노선 펨토초 레이저 조사에 의해 유도되는 전자기장 및 온도장 수치 해석

  • Ha, Jeonghong (Department of Mechanical Engineering, Pohang University of Science and Technology (POSTECH)) ;
  • Kim, Dongsik (Department of Mechanical Engineering, Pohang University of Science and Technology (POSTECH))
  • 하정홍 (포항공과대학교 기계공학과) ;
  • 김동식 (포항공과대학교 기계공학과)
  • Received : 2015.03.06
  • Accepted : 2015.03.25
  • Published : 2015.03.31

Abstract

This work performed numerical analysis of electromagnetic field and thermal phenomena occurring in femtosecond laser irradiation of silver nanowires. The local electric field enhancement was computed to calculate the optical energy dissipation as a Joule heating source and the thermal transport was analysed based on the two-temperature model (TTM). Electron temperature increased up to 1000K after 50fs and its spatial distribution became homogeneous after 80fs at the fluence of 100mJ/cm2. The result of this work is expected to contribute to revealing the photothermal effects on silver nanowires induced by femtosecond laser irradiation. Although the highest increase of lattice temperature was substantially below the melting point of silver, the experimental results showed resolidification and fragmentation of the silver nanowire into nanoparticles, which cannot be explained by the photothermal mechanism. Further studies are thus needed to clarify the physical mechanisms.

Keywords

References

  1. S. De, T.M. Higgins, P.E. Lyons, E.M. Doherty, P.N. Nirmalraj, W.J. Blau, J.J. Boland, and J.N. Coleman, "Silver nanowire networks as flexible, transparent, conducting films: extremely high DC to optical conductivity ratios," ACS Nano, 3(7), 1767-1774. (2009) https://doi.org/10.1021/nn900348c
  2. D.S. Hecht, L. Hu, and G. Irvin, "Emerging transparent electrodes based on thin films of carbon nanotubes, graphene, and metallic nanostructures," Adv. Mater. 23 (2011)
  3. D.S. Hecht, and R.B. Kaner, "Solution-processed transparent electrodes," MRS Bull. 36 (2011)
  4. K. Ellmer, "Past achievements and future challenges in the development of optically transparent electrodes," Nat. Photon. 6 (2012)
  5. J.Y. Lee, S.T. Connor and Y. Cui, "Solutionprocessed metal nanowire mesh transparent electrodes," Nano Lett. 8 (2008)
  6. T. Tokuno, M. Nogi, M. Karakawa, J. Jiu, T. T. Nge, Y. Aso, and K. Suganuma, "Fabrication of silver nanowire transparent electrodes at room temperature," Nano Res. 4 (2011)
  7. T.B. Song, Y. Chen, C.H. Chung, Y. Yang, B. Bob, H.S. Duan, G. Li, K. Tu, Y. Huang, and Y. Yang, "Nanoscale Joule heating and electromigration enhanced ripening of silver nanowire contacts," ACS Nano 8 (2014)
  8. H. Wu, L. Hu, M.W. Rowell, D. Kong, J. J. Cha, J.R. McDonough, J. Zhu, Y. Yang, M.D. McGehee, and Y. Cui, "Electrospun metal nanofiber webs as high-performance transparent electrode," Nano Lett. 10 (2010)
  9. E.C. Garnett, W. Cai, J.J. Cha, F. Mahmood, S.T. Connor, M.G. Christoforo, Y. Cui, M.D. McGehee, and M.L. Brongersma, "Self-limited plasmonic welding of silver nanowire junctions," Nat. Mater. 11 (2012)
  10. L.O. Herrmann, V.K. Valev, C. Tserkezis, J.S. Barnard, S. Kasera, O.A. Scherman, J. Aizpurua, and J.J. Baumberg, "Threading plasmonic nanoparticle strings with light," Nat. Comm. 5 (2014)
  11. H. Huang, L. Liu, P. Peng, A. Hu, W.W. Duley, Y. Zhou, "Controlled joining of Ag nanoparticles with femtosecond laser irradiation," J. Appl. Phys. 112 (2012)
  12. Z. Du, C. CHen, L. Traverso, X. Xu, and L. Pan, "Optothermal response of plasmonic nanofocusing lens under picosecond laser irradiation," Proc. of SPIE 8967 (2014)
  13. E.D. Palik, Handbook of Optical Constants of Solids (Academic, 1985), Vol. 1, p. 50.
  14. Z. Lin, L.V. Zhigilei, and V. Celli, "Electronphonon coupling and electron heat capacity of metals under conditions of strong electron-phonon nonequilibrium," Phys. Rev. B 77 (2008)
  15. David R. Lide (ed), CRC Handbook of Chemistry and Physics, 84th Edition. (CRC Press. Boca Raton, Florida, 2003)
  16. W.W. Duley, UV Lasers: Effects and Applications in Materials Science (Cambridge University Press, New York, 1996), p. 67.
  17. S.D. Brorson, J.G. Fujimoto, and E.P. Ippen, "Femtosecond electronic heat-transport dynamics in thin gold films," Phys. Rev. Lett. 59 (1987)
  18. T. Juhasz, H. E. Elsayed-Ali, G.O. Smith, C. Suarez, and W. E. Bron, "Direct measurements of the transport of nonequilibrium electrons in gold films with different crystal structures," Phys. Rev. B 48 (1993)