Bulletin of the Korean Chemical Society

Korean Chemical Society (대한화학회)
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A Novel 3D Polypseudo-rotaxane Metal-organic Framework Based on a Flexible Bis-pyridyl-bis-amide Ligand

  • Wang, Xiu-Li (Department of Chemistry, Bohai University) ;
  • Han, Na (Department of Chemistry, Bohai University) ;
  • Lin, Hong-Yan (Department of Chemistry, Bohai University) ;
  • Xu, Chuang (Department of Chemistry, Bohai University) ;
  • Luan, Jian (Department of Chemistry, Bohai University) ;
  • Liu, Guo-Cheng (Department of Chemistry, Bohai University)
  • Received : 2012.08.01
  • Accepted : 2012.08.30
  • Published : 2012.11.20
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Abstract

A novel 3D compound $\{[Cu(L)(H_2O)_4][Cu_2(SIP)_2(L)_2]\}{\cdot}2H_2O$ (1) (L = N,N-bis(4-pyridinecarboxamide)-1,4-butane, SIP = 5-sulfoisophthalate) is hydrothermally synthesized. X-ray diffraction analysis reveals that compound 1 is composed of 2D anionic $[Cu_2(SIP)_2(L)_2]_n{^{2n-}}$ double-layers and discrete 1D cationic $[CuL(H_2O)_4]_n{^{2n+}}$ polymeric chains, which represents a rare 3D polypseudo-rotaxane MOF from intercalation of 1D and 2D framework. In addition, the luminescent property and electrochemical behavior of compound 1 have been investigated.

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References

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