Nuclear Engineering and Technology

  • 제41권7호
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  • Pages.979-988
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  • 2009
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  • 1738-5733(pISSN)
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  • 2234-358X(eISSN)
한국원자력학회 (Korean Nuclear Society)
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NEUTRON-INDUCED CAVITATION TENSION METASTABLE PRESSURE THRESHOLDS OF LIQUID MIXTURES

  • Xu, Y. (School of Nuclear Engineering, Purdue University) ;
  • Webster, J.A. (School of Nuclear Engineering, Purdue University) ;
  • Lapinskas, J. (School of Nuclear Engineering, Purdue University) ;
  • Taleyarkhan, R.P. (School of Nuclear Engineering, Purdue University)
  • 발행 : 2009.09.30
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초록

Tensioned metastable fluids provide a powerful means for low-cost, efficient detection of a wide range of nuclear particles with spectroscopic capabilities. Past work in this field has relied on one-component liquids. Pure liquids may provide very good detection capability in some aspects, such as low thresholds or large radiation interaction cross sections, but it is rare to find a liquid that is a perfect candidate on both counts. It was hypothesized that liquid mixtures could offer optimal benefits and present more options for advancement. However, not much is known about radiation-induced thermal-hydraulics involving destabilization of mixtures of tensioned metastable fluids. This paper presents results of experiments that assess key thermophysical properties of liquid mixtures governing fast neutron radiation-induced cavitation in liquid mixtures. Experiments were conducted by placing liquid mixtures of various proportions in tension metastable states using Purdue's centrifugally-tensioned metastable fluid detector (CTMFD) apparatus. Liquids chosen for this study covered a good representation of both thermal and fast neutron interaction cross sections, a range of cavitation onset thresholds and a range of thermophysical properties. Experiments were devised to measure the effective liquid mixture viscosity and surface tension. Neutron-induced tension metastability thresholds were found to vary non-linearly with mixture concentration; these thresholds varied linearly with surface tension and inversely with mixture vapor pressure (on a semi-log scale), and no visible trend with mixture viscosity nor with latent heat of vaporization.

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참고문헌

  1. R. Akasaka, T. Yamaguchi, T. Ito, “Practical and direct expressions of the heat of vaporization for mixtures”, Chemical Engineering Science, 60, pp. 4369-4376, 2005 https://doi.org/10.1016/j.ces.2005.03.005
  2. R. E., Apfel, “The superheated drop detector,” Nuclear Instruments and Methods, Vol.162, Issues 1-3, pp. 603-608, June (1979) https://doi.org/10.1016/0029-554X(79)90735-3
  3. C. R. Bell, N. P. Oberle, W. Rohsenow, N. Todreas, and C. Tso, “Radiation-Induced Boiling in Superheated Water and Organic Liquids,” Nuclear Science and Engineering, Vol.53, pp. 458-465, (1974) https://doi.org/10.13182/NSE74-A23376
  4. Chemical properties handbook, online at http://www.knovel.com/knovel2
  5. R. M. Digilov, M. Reiner, "Weight-controlled capillary viscometer", AM. J. Phys., Vol. 73, No. 11, pp. 1020-1022, Nov. (2005) https://doi.org/10.1119/1.2060718
  6. E. Forringer, D. Robbins, J. Martin, “Confirmation of Neutron Production During Self-Nucleated Acoustic Cavitation”, Proc. Amer. Nucl. Soc., 736-737, Nov., (2006)
  7. D. A. Glaser, “The bubble chamber,” Encyclopedia of Physics, 316-341, Nuclear Instrumentation II. S. Fluggeld, Springer-Verlag, (1958)
  8. M. Greenspan, C. E. Tschiegg, “Radiation-induced acoustic cavitation; threshold versus temperature for some liquids”, J. Acoustic Soc. Am., Vol.74, no.4, pp.1327-1331, Oct., (1982) https://doi.org/10.1121/1.388415
  9. B. Hahn, “The fracture of liquids under stress due to ionizing particles”, Nuovo Cimento, Vol. 22, pp. 650-653, (1961) https://doi.org/10.1007/BF02774902
  10. H. Ing, R. A. Noulty, and T. D. McLean, “Bubble detectors- A maturing technology”, Radiation Measurements, Vol. 27, Issue 1, pp. 1-11, Feb. (1997) https://doi.org/10.1016/S1350-4487(96)00156-4
  11. J. Kendall and K.P. Monroe, “The Viscosity of Liquids. II. The Viscosity-Composition Curve for Ideal Liquid Mixtures”, J. Am. Chem. Soc. Vol. 39, No. 9, pp. 1787-1806, 1917 https://doi.org/10.1021/ja02254a001
  12. R. T. Lahey, R. P. Taleyarkhan, R. I. Nigmatulin and I. Akhatov, “Sonoluminescence and the search for Sonofusion”, Adv. in Heat Transfer, Vol. 39, (2006) https://doi.org/10.1016/S0065-2717(06)39001-6
  13. J. Lapinskas, P. Smagacz, J. Webster, P. Shaw, Y. Xu and R. P. Taleyarkhan, “Fast Neutron Gamma-Insensitive Continuous Operation Tension Metastable Fluid Detector,” Transac. Proc. Amer. Nucl. Soc. Conf., Reno, NV, (2006)
  14. D. Lieberman, “Radiation-induced cavitation”, The Physics of Fluids, Vol.2, No.4, pp. 466-468, July-Aug., (1959) https://doi.org/10.1063/1.1724419
  15. R. A. McAllster, “The Viscosity of Liquid Mixtures,” AIChE Journal, Vol.6, No.3, pp. 427-431, (1959) https://doi.org/10.1002/aic.690060316
  16. R. I. Nigmatulin, I. Akhatov, A. Topolinokov, R. Bolotnova, N. Vakhitova, R. T. Lahey, Jr. and R. P. Taleyarkhan, “Theory of supercompression of vapor bubbles and nanoscale thermonuclear fusion”, Phys. of Fluids, Vol.17, 107106, (2005) https://doi.org/10.1063/1.2104556
  17. D. Santrach and J. Lielmezs, “The latent heat of vaporization prediction for binary mixtures”, Industrial Engineering Chemical Fundamentals, Vol. 17, No. 2, pp. 93-96, 1978 https://doi.org/10.1021/i160066a004
  18. F. Seitz, “On the theory of the bubble chamber,” The Physics of Fluids, Vol.1, No.1, pp. 2-13, January-February, (1958) https://doi.org/10.1063/1.1724333
  19. P. Smagacz, J. Lapinskas, A. Horn, Y. Xu and R. P. Taleyarkhan, “Fast Neutron Gamma-Insensitive Centrifugally-Tensioned Metastable Fluid Detector,” Transac. Proc. Amer. Nucl. Society, Reno, NV, (2006)
  20. R. P. Taleyarkhan, C. D. West, J. Cho, R. T. Lahey, Jr., R. I. Nigmatulin and R. C. Block, “Evidence of nuclear emissions during acoustic cavitation,” Science, Vol. 295, (2002) https://doi.org/10.1126/science.295.5562.2002
  21. R. P. Taleyarkhan, J. Cho, C. D. West, R. T. Lahey, Jr., R. I. Nigmatulin and R. C. Block, “Additional Evidence of nuclear emissions during acoustic cavitation,” Phys. Rev. E., (2004) https://doi.org/10.1103/PhysRevE.63.036109
  22. R. P. Taleyarkhan, C. D. West, R. T. Lahey, Jr., R. I. Nigmatulin, R. C. Block, and Y. Xu, “Nuclear emissions during self-nucleated acoustic cavitation,” Phys. Rev. Ltrs., (2006) https://doi.org/10.1103/PhysRevLett.96.034301
  23. A. Tamir, “Correlations for predicting azeotropic heat of vaporization of multicomponent mixtures,” Ind. Eng. Chem. Fundam., Vol.22, No.1, pp. 83-86, (1983) https://doi.org/10.1021/i100009a014
  24. Y. Xu, and A. Butt, “Confirmation of nuclear emissions during acoustic cavitation,” Nuclear Engineering and Design, Vol. 235, pp. 1317-1324, (2005) https://doi.org/10.1016/j.nucengdes.2005.02.021
  25. Y. Xu, P. Smagacz, J. Lapinskas, J. Webster, P. Shaw and R. P. Taleyarkhan, “Neutron Detection with Centrifugally-Tensioned Metastable Fluid Detectors,” ICONE-14, Miami, Florida, USA, July 17-20, (2006)