Application of Representative $PM_{2.5}$ Source Profiles for the Chemical Mass Balance Study in Seoul

  • Kang, Choong-Min (Exposure, Epidemiology and Risk Program, Harvard School of Public Health, USA) ;
  • Kang, Byung-Wook (Division of Environmental Engineering, Chungju National University) ;
  • SunWoo, Young (Department of Environmental Engineering, Konkuk University) ;
  • Lee, Hak-Sung (Department of Environmental, Civil and Information System, Seowon University)
  • Published : 2008.06.30

Abstract

Source samples were collected to construct source profiles for 9 different source types, including soil, road dust, gasoline/diesel-powered vehicles, a municipal incinerator, industrial sources, agricultural/biomass burning, marine aerosol, and a coal-fired power plant. Seasonal profiles for 'Chinese aerosol', aerosols derived from the urban area of China, were reconstructed from seasonal $PM_{2.5}$ compositions reported in Beijing, China. Ambient $PM_{2.5}$ at a receptor site was also measured during each of the four seasons, from April 2001 to February 2002, in Seoul. The Chemical Mass Balance receptor model was applied to quantify source contributions during the study period using the estimated source profiles. Consequently, motor vehicle exhaust (33.0%), in particular 23.9% for diesel-powered vehicles, was the largest contributor affecting the $PM_{2.5}$ levels in Seoul, followed by agricultural/biomass burning (21.5%) and 'Chinese aerosol' (13.1%), indicating contributions from long-range transport. The largest contributors by season were: for spring, 'Chinese aerosol' (31.7%); for summer, motor vehicle exhaust (66.9%); and for fall and winter, agricultural/biomass burning (31.1% and 40.1%, respectively). These results show different seasonal patterns and sources affecting the $PM_{2.5}$ level in Seoul, than those previously reported for other cities in the world.

Keywords

References

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