Adsorptive Catalytic Wave of Chromium-Cupferron Complex

크롬-쿠페론 착물의 흡착 촉매파

  • Received : 2002.01.24
  • Published : 2002.06.25

Abstract

The interfacial accumulation of the chromium-cupferron complex and the catalytic wave of its redox process is characterized by cyclic voltammetry. One cathodic peak is observed in the forward scan at -1.45 V. Scanning in the reverse direction produces a inverted peak at -1.39 V, which is indicative of a catalytic process. The optimal conditions of inverted peak were found to be 1 mM borate buffer solution(pH 9.48) containing $1{\times}10^{-4}M$ cupferron, holding potential of -1.8 V and scan rate of 20 mV/s. Using main peak, a preconcentration time of 1 min results in a detection limit of $3.2{\times}10^{-10}M$.

크롬-쿠페론착물의 표면 축적과 촉매 특성을 순환 전압전류법으로 조사하였다. 정 방향으로 주사할 때에 -1.45 V에서 환원 봉우리가 생기고 역 주사할 때에 -1.39 V에서 반전된 봉우리가 생기는데 이는 촉매과정을 나타낸다. 이 반전 봉우리의 최적 실험 조건은 $1{\times}10^{-4}M$ 쿠페론이 포함된 붕산염 완충용액(pH 9.48), 축적전위 -1.8 V, 주사속도 20 mV/s이었다. 이 조건에서 주 봉우리를 이용하여(축적시간 1분) 얻은 크롬의 검출한계는 $3.2{\times}10^{-10}M$이다.

Keywords

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