Neutron Cross Section Evaluation on Mo-95, Tc-99, Ru-101 and Rh-1()3 in the Fast Energy Region

  • Lee, Y. D. (Korea Atomic Energy Research Institute) ;
  • J. H. Chang (Korea Atomic Energy Research Institute)
  • Published : 2002.12.01

Abstract

The neutron induced nuclear data for Mo-95, Tc-99, Ru-101 and Rh-103 was calculated and evaluated in the fast energy region. The energy dependent optical model potential parameters were extracted based on the recent experimental data and applied up to 20 MeV. The s-wave strength function was calculated from the parameters. Spherical optical model, statistical model in equilibrium energy, multistep direct and multistep compound model in pre-equilibrium energy and direct capture model were used in the calculation. The theoretically calculated cross sections were compared with the experimental data and the evaluated files The model- calculated total and capture cross sections were in good agreement with the reference experimental data. The direct capture contribution improved the capture cross sections in pre- equilibrium region. The evaluated cross section results were compiled to ENDF-6 format and will improve the ENDF/B-Vl.

Keywords

References

  1. J.H. Chang et al., Establishment of Nuclear Data System, KAERI/RR-2121/(2000)
  2. Y.D. Lee and J.H. Chang, 'Neutron Cross Section Evaluation on Pr-141, Nd-143, Nd-145, Sm-147, Sm-149,' J. of KNS to be published, (2002)
  3. S.Y.Oh and J.H.Chang, Neutron Cross Section Evaluations of Fission Products below the Fast Energy Region, BNL-NCS-67496 (KAERI/TR-1511/2000), Brookhaven National Laboratory
  4. P.F. Rose, Ed., 'ENDF/B-VI Summary Documentation,' BNL-NCS-17541 (ENDF-201), National Nuclear Data Center, BNL, (1991)
  5. M.Herman, Empire-II: Statistical Model Code for Nuclear Reaction Calculations, IAEA, (2000)
  6. S. Igarasi, Optical Model Potentials used in JENDL Evaluations (JAERI, Tokaimura, Japan), Reference Input Parameter Library for theoretical calculations of nuclear reactions (RIPL), JAERI 1228(41), (1973)
  7. R.D.Lawsonm ABAREX_A Neutron Spherical Optical-Statistical Model Code, in Workshop on Computation and Analysis of Nuclear Data Relevant to Nuclear Energy and Safety, pp447, Trieste, Italy
  8. T. Nakagawa, et al., Japanese Evaluated Nuclear Data Library, Version 3, Revision 2, J. Nucl. Sci. Technol. 32, 1259, (1995)
  9. A. Gilbert and A.G.W. Cameron, Can. J. Phys. 43, 1446, (1965)
  10. A.V. Ignatyuk, G.N. Smirenkin and A. S. Tishin, Sov. J. Nucl. Phys. 21, 255, (1975)
  11. M.V. Pasechnik et al., 'Total Neutron Cross Sections for Molybdenum and Zyrconium at Low Energies,' C, 80KIEV, 1, 304, (1980)
  12. A.R.DEL.Musgrove et al., 'Average Neutron Resonance Parameters and Radiative Capture Cross Sections for the Isotopes of Molybdenum,' J, NP/A, 270, 108, (1976)
  13. D.G.Foster JR, D.W. Glasgon, 'Neutron Total Cross Sections, 2.5 - 15 MeV,' J, PR/C, 3, 576, (1971)
  14. R.L. Macklin, 'Technetium-99 Neutron Capture Cross Section,' J, NSE, 81, 520, (1982)
  15. S.M. Qaim, 'Nuclear Reactions Cross-Sections for 14.7 MeV Neutrons on TC-99,' J, JIN, 35, 3669, (1973)
  16. R. W. Hockenbury, 'Capture Cross sections of 145-Nd, 149-Sm, 101-Ru, 102-Ru, and 104-Ru,' Bull. Amer. Phys. Soc., Vol.20, pp560, (1975)
  17. M.V. Bokhovko et al., 'Neutron Radiation Cross-Section, Neutron Transmission And Average Resonance Parameters For Some Fission Product Nuclei,' R, FEI-2168-91, (1991)