Three-dimensional numerical simulation of nonisothermal coextrusion process with generalized Newtonian fluids

  • Sunwoo, Ki-Byung (School of Chemical Engineering, Seoul National University) ;
  • Park, Seung-Joon (School of Chemical Engineering, Seoul National University) ;
  • Lee, Seong-Jae (Department of Polymer Engineering, The University of Suwon) ;
  • Ahn, Kyung-Hyun (School of Chemical Engineering, Seoul National University) ;
  • Lee, Seung-Jong (School of Chemical Engineering, Seoul National University)
  • Published : 2000.12.01

Abstract

Three-dimensional numerical simulation of isothermal/nonisothermal coextrusion process of two immiscible polymers through a rectangular channel has been done using the finite element method. The encapsulation phenomenon with the less viscous layer encapsulating the more viscous layer was investigated with the generalized Newtonian fluids. The interface position around the symmetric plane obtained by numerical simulation nearly coincided with the one observed in experiments, but the degree of encapsulation was less than the one observed experimentally. Open boundary condition method was found to be applied to the simulation of nonisothermal coextrusion process, however, the results are not far from those using the fully developed boundary condition, because the temperature development along the downstream direction is very slow in the case of convection dominated flow. When the inlet velocity is increased, the interface profile does not change in isothermal flow, while it moves upward in nonisothermal situation. The degree of encapsulation decreases along the downstream direction in nonisothermal flow. When the inlet temperature increases compared to the wall temperature, the outlet interface moves downward and the degree of encapsulation increases. The difference of degree of encapsulation between the simulation and the experiments seems to arise from the viscoelastic effect of the materials. It was concluded that the nonisothermal effect alone does not explain the complex coextrusion process and the viscoelastic effect needs to be considered.

Keywords

References

  1. Polym. Eng. Sci. v.34 Prediction of stationary interfaces in Coextrusion flows Agassant J. F.;A. Fortin
  2. Polym. Eng. Sci. v.37 A three-dimensional analysis of coextrusion Gifford W. A.
  3. J. Appl. Polym. Sci. v.17 A. study of bicomponent coextrusion of molten polymers Han C. D.
  4. J. Appl. Polym. Sci. v.20 Further observations of the interface shape of conjugate fibers Han C. D.;Y. W. Kim
  5. Rheol. Acta. v.29 Three-dimensional studies on bicomponent extrusion Karagiannis A.;A. N. Hrymak;J. Vlachopoulos
  6. Trans. Soc. Rheol. v.18 An experimental study of rheological properties of polymer melts in laminar shear flow and interface deformation and its mehanism in two-phase stratified flow Lee. B. L.;J. L. White
  7. Kor. J. Rheol. v.2 Numerical prediction of three dimensional extrudate swell Lee S. J.;S. J. Lee
  8. AIChE J. v.33 Finite element simulation of stratified multiphase flows Mavridis H.;A. N. Hrymak;J. Vlachopoulos
  9. Polym. Eng. Sci. v.15 Co-extrusion of unfilled and TiO2-filled polyethylene: Influence of viscosity and die cross-section on interface shape Minagawa N.;J. L. White
  10. J. Non-Newtonian Fluid Mech. v.87 On the use of the open boundary condition method in the numerial simulation of nonisothermal viscoelastic flow Park S. J.;S. J. Lee
  11. J. Polym. Sci. v.13 Additional observations on stratified bicomponent flow of polymer melts in a tube Southern J. H.;R. L. Ballman
  12. J. Non-Newtonian Fluid Mech. Numerical simulation of three-dimensional viscoelastic flow using the open boundary condition method in coextrusion process Sunwoo K. B.;S. J. Park;S. J. Lee;K. H. Ahn;S. J. Lee
  13. Rheol. Acta v.37 Three-dimensional viscoelastic numerial analysis of the encapsulation phenomena in coextrusion Takase M.;S. Kihara;K. Funatsu
  14. Rheol. Acta. v.32 Boundary conditions for contact lines in coextrusion flows Torres A.;A. N. Hrymak;J. Vlachopoulos;J. Dooley;B. T. Hilton