Journal of Korean Society for Atmospheric Environment (한국대기환경학회지)

Korean Society for Atmospheric Environment (한국대기환경학회)
권호 표지

Seasonal Variation of Size Distributions of Polycyclic Aromatic Hydrocarbons in Air Particulates

대기 부유분진중 다환방향족 탄화수오류의 계절적 입경농도 분포 변이

  • Chung, Yong (Institute for Environmental Research, Yonsei University) ;
  • Park, Seong-Eun (Institute for Environmental Research, Yonsei University) ;
  • Hwang, Man-Sik (Institute for Environmental Research, Yonsei University)
  • 정용 (연세대학교 환경공해연구소) ;
  • 박성은 (연세대학교 환경공해연구소) ;
  • 황만식 (연세대학교 환경공해연구소)
  • Published : 1998.12.01
Download PDF
⟨ Previous Next ⟩

Abstract

Polycyclic aromatic hydrocarbons (PAHs) are products of incomplete combustion and, in urban area atmosphere, are mainly traffic or heating in origin. Size-segregated aerosol samples were collected on the Eixth story of Shinchon on the Yonsei campus, using a high-volume cascade impactor, between August 1994 and September 1995. Ten PAHs were analyzed by GC/MSD. The size distribution of PAH-containing particulates followed approximately a log-normal relationship with the majority of PAH content associated with particles below 3.0mm. PAHs concentration in submicron particles increased during the winter months. The Mass Median Diameter (MMD) value of annual particulates in the heavy traffic area of Shinchon shows about 1.6 pm. The MMD values of air particulate in winter were the lowest values and similar to that in summer, while MMD values of seasonal PAHs were generally lower than 1.0 pm. Among the PAHs, MMD values of PAHs with the more than 5 benzen ring were averagely lower than those with 4 benzin rings. Especially MMD's of dibenzo (a, h) anthracene in winter was clearly lower than in summer. This reason may be caused by fuels used for heating. In this area, 50∼80% PAHs mass was particles smaller than 1.0mm aerodynamic diameter in size range, and the MMD values of PAHs lower than those of other country's area.

Keywords

References

  1. 한국대기보전학회지 v.8 no.40 서울시 대기부유분진의 농도와 다환 방향족 유기물질에 의한 발암위해성 박성은;정용
  2. 대한 환경공학회지 v.18 환경대기 중 다환방향족 탄화수소의 출현양상과 거동(Ⅰ) - 지역적 및 계절적 농도분포 백성옥;최진수
  3. 한국대기보전학회지 v.2 no.3 대기 중 중금속의 입경분포에 관한 연구 손동헌;강춘원
  4. 한국대기보전학회지 v.12 no.1 대기부유분진중 미량 금속 원소의 입경별 농도분포에 관한 연구 신훈중;이태정;김동술
  5. 한국대기보전학회지 v.4 no.2 황사현상이 분진의 입도분포와 화학조성에 관한 연구 이민희;한의정;원양수
  6. 한국대기보전학회지 v.1 Andersen 시료채취기를 이용한 도시대기 중 부유입자상 물질의 입도분포 측정 이용근;김만구;원정호
  7. 한국대기보전학회지 v.13 no.4 수원지역 입자상 오염물질의 오염원 기여도의 추정 이태정;김동술
  8. 한국대기보전학회지 v.5 no.1 호흡성 분진중의 중금속 오염도에 관한 조사연구 임영욱;정용
  9. 환경성 발암원 돌연변이학회지 v.15 no.2 대기 부유분진중 발암성 유기추출물의 화학적 조성 및 돌연변이원성 정용;신동천;박성은;황만식;이현
  10. 한국대기보전학회지 v.10 no.1 도시대기부유분진중 다환방향족 탄화수소의 농도 및 입경 분포 특성 조기철;이승일;김달호;허귀식;김희강
  11. 한국대기보전학회지 v.13 no.1 도시 대기 중에 부유하는 미세입자중 음이온의 농도분포 특성 천만영;조기철;여현구
  12. 예방의학회지 v.19 no.1 한 도시 분진의 유해성 입도 분포에 대한 조사 연구 한의정;정용;권숙표
  13. 환경백서 환경부
  14. Environ. Lett. v.6 Size-distribution pattern of polycyclic aromatic hydrocarbons in airborne particulates Albagli, A.;H. Oja;L. Dubois
  15. Handbook of Polycyclic Aromatic Hydrocarbons Bjorseth, A.(Ed.)
  16. Atmos. Environ. v.12 Any factors influencing the dispersion and the transport of heavy hydrocarbons associated with airborne particles De Wiest, F.
  17. J. Air Pollut. Contr. Assoc. v.16 Polynuclear aromatic hydrocarbons associated with Particulates in Pittsburgh Air Demaio, L.;M. Corn
  18. Environmental Carcinogens: Polycyclic Aromatic Hydrocarbons Grimmer, G.(Ed.)
  19. Aerosol. Sci. Technol. v.14 Hildemann, L.M.;G.R. Markowski;M.C. Jones;G.R. Cass
  20. Environmental Science & Technology v.14 no.7 Comparative distribution of eight polycyclic aromatic hydrocarbons in airborne particulates collected by conventional high-volume sampling and by size fractionation Kartz, M.;C. Chan
  21. Atmos. Environ. v.5 On the size distribution on benzo(a)pyrene containing particles in urban air Kertesz-SDaringer, M.;E. Meszaros;T. Varkonyi
  22. JAPCA v.28 no.4 Summary of the New York summer aerosol study (NASAS) Leaderer, BP.;DM Bernstein;JM. Daisey;MT. Kleinman;TJ. Kneip;EO. Knutson;M. Lippman;PY. Lioy;KA Rahn;D. Sinclair;RL. Tanner;GT. Wolff
  23. Science v.178 The size of suspended particulate matter in air Lee, R.E.
  24. The Science of the Total Environment v.116 Urban air pollution by polycyclic aromatic hydrocarbons: Levels and sources of variability Menichini, E.
  25. Polycyclic Aromatic Hydrocarbons: Evaluation of Sources and Effects National Academy Science
  26. Science v.41;186 no.65 Urban aerosol toxicity: The influence of particle size Natuch, D.F.S.;J.R. Wallace
  27. Mut. Res. v.276 Mutagenicity studies on complex environmental mixtures: selection of solvent system for extraction Nielsen, P.A.
  28. Manual of Analytical Method NIOSH
  29. Polycyclic Aromatic Hydrocarbons National Research Council
  30. Environmental Science & Technology v.9 no.4 Dependency of polynuclear aromatic hydrocarbon content on size distribution of Atmospheric aerosols Pierce, R.C.;K. Morris
  31. J. Nat. Cancer Inst. v.33 Experimentl studies of the conditions of exposure to carcinogens for lung cancer induction Saffiotti, U.;F. Cefis;L.H. Kolb;P. Shubik
  32. Health and Ecological Assessment of Polycyclic Aromatic Hydrocarbons Santodonato, J.;P. Howard;D. Basu
  33. EPA/600/P-95/ø ø 1bF v.1 Air Quality Criteria for Particulate Matter US EPA
  34. Aerosols, Research, Risk Assessment and Control Strategies Sampling, size distribution, reactivity and analysis of organic aerosol constituents Van, C.K.;Lee S.D.(et al)(Eds)
  35. Environmental Science and Technology v.28 Size distributions of polycyclic aromatic hydrocarbons and elemental carbon. 1. Sampling, Measurement Methods, and Source Characterization Venkartaraman, C.;J.M. Lyons;S.K. Friedlander
  36. J. of colloid and interface Science v.39 The aerosol size distribution of Los angeles Smog Whitby, K.T.;R.B. Husar;B.Y.H. Liu
  37. WHO Reg. Pub., Eur., Series No. 23 Polynuclear Aromatic Hydrocarbons (PAHs), In Air Quality Guidenline for Europe WHO