Thermal Behavior and Degradation Mechanism of Aromatic Polyester Polymer

방향족 폴리에스테르의 열적거동과 분해 반응 기구

  • 박상순 (한양대학교 공과대학 섬유공학과) ;
  • 김동국 (한양대학교 이과대학 화학과, 한양대학교 공과대학 섬유공학과) ;
  • 임승순
  • Published : 1994.03.01

Abstract

Thermal analysis has been carried out on aromatic polyesters(i.e. poly(ethylene 2,6-naphlhalate) and poly(butylene 2,6-naphthalate)) over a range of 270 to 31$0^{\circ}C$, above the melting temperature, without the addition of catalysts and stabilizers. Degradation products of polyesters were characterized by gas chromatography and mass spectrometer. It was concluded that poly(ethylene 2,6-naphthalate) decomposed by a random scission of ester links involving a six centered cyclic transition state yields vinyl naphthoate and naphthoic acid and poly(butylene 2,6-naphthalate) decomposed by two random scission of ester links gives 1-butenyl naphthoate and naphthoic acid.

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