Ultra-Clean Patterned Transfer of Single-Layer Graphene by Recyclable Pressure Sensitive Adhesive Films

  • Kim, Sang Jin (Institute of Advanced Composite Materials, Korea Institute of Science and Technology) ;
  • Lee, Bora (Department of Chemistry, Seoul National University) ;
  • Choi, Yong Seok (Department of Chemistry, Seoul National University) ;
  • Kim, Philip (Department of Physics, Harvard University) ;
  • Hone, James (Department of Mechanical Engineering, Columbia University) ;
  • Hong, Byung Hee (Department of Chemistry, Seoul National University) ;
  • Bae, Sukang (Institute of Advanced Composite Materials, Korea Institute of Science and Technology)
  • Published : 2016.02.17

Abstract

We report an ultraclean, cost-effective, and easily scalable method of transferring and patterning large-area graphene using pressure sensitive adhesive films (PSAFs) at room temperature. This simple transfer is enabled by the difference in wettability and adhesion energy of graphene with respect to PSAF and a target substrate. The PSAF transferred graphene is found to be free from residues, and shows excellent charge carrier mobility as high as ${\sim}17,700cm^2/V{\cdot}s$ with less doping compared to the graphene transferred by thermal release tape (TRT) or poly(methyl methacrylate) (PMMA) as well as good uniformity over large areas. In addition, the sheet resistance of graphene transferred by recycled PSAF does not change considerably up to 4 times, which would be advantageous for more cost-effective and environmentally friendly production of large-area graphene films for practical applications.

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